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JAEA Reports

Training using JMTR and related facilities in FY2021 and FY2022

Nakano, Hiroko; Fujinami, Kyoko; Yamaura, Takayuki; Kawakami, Jun; Hanakawa, Hiroki

JAEA-Review 2023-036, 33 Pages, 2024/03

JAEA-Review-2023-036.pdf:2.47MB

A practical training course using the JMTR (Japan Materials Testing Reactor) and other research infrastructures was held from November 29 to December 2 in 2021 for Asian young researchers and engineers. This course was adopted as International Youth Exchange Program in Science (SAKURA SCIENCE Exchange Program) which is the project of the Japan Science and Technology Agency, and this course aims to enlarge the number of high-level nuclear researchers/engineers in Asian countries which are planning to introduce a nuclear power plant, and to promote the use of facilities in future. In this year, from the viewpoint of preventing the spread of COVID-19 infection, it was decided to hold the event online. 53 young researchers and engineers joined the course from 6 countries. In FY2022, training programs with invitations were held due to the easing of restrictions on entry into Japan from overseas. 7 young researchers and engineers from4 Asian countries participated in the training from February 1 to 10, 2023.The common curriculum in the training course of FY2021 and FY2022 included lectures on nuclear energy, irradiation testing, safety management, JMTR decommissioning plan, etc. In the online session, conducted in FY2021, information exchange on the energy situation in each country was conducted. On-site training conducted in FY2022, included practical training on operation using simulations, environmental monitoring, etc. and facility tours of the JMTR, etc. Many participants could join the online training course, they created a diversity of expertise and made lively discussions during the information exchange. On-site training, while limited in number of participants, provided a good opportunity for personnel exchange through practical training and face-face communication. It is desirable to hold on-site training as long as circumstances permit. This report summarizes the training conducted in FY2021 and FY2022.

Journal Articles

The Role of collision ionization of K-shell ions in nonequilibrium plasmas produced by the action of super strong, ultrashort PW-class laser pulses on micron-scale argon clusters with intensity up to 5 $$times$$ 10$$^{21}$$ W/cm$$^{2}$$

Skobelev, I. Yu.*; Ryazantsev, S. N.*; Kulikov, R. K.*; Sedov, M. V.*; Filippov, E. D.*; Pikuz, S. A.*; Asai, Takafumi*; Kanasaki, Masato*; Yamauchi, Tomoya*; Jinno, Satoshi; et al.

Photonics (Internet), 10(11), p.1250_1 - 1250_11, 2023/11

 Times Cited Count:0 Percentile:0(Optics)

It is challenging to clearly distinguish the impacts of the optical field and collisional ionization in the evolution of the charge state of a plasma produced when matter interacts with high-intensity laser pulses. In this work, time-dependent calculations of plasma kinetics are used to show that it is possible only when low-density gaseous targets with sufficiently small clusters are used. In the case of Ar plasma, the upper limit of the cluster radius was estimated to be $$R_0 = 0.1 mu$$m.

Journal Articles

Band gap formation in graphene by hybridization with Hex-Au(001) reconstructed surface

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Vacuum and Surface Science, 66(9), p.525 - 530, 2023/09

As Au (001) surfaces exhibit a quasi-one-dimensional corrugated structure, Hex-Au(001), its periodicity was predicted to change the electronic structure of graphene when graphene was grown on this surface. Furthermore, the hybridization between graphene and Au is known to introduce bandgap and spin polarization into graphene. Here, we report angle-resolved photoemission spectroscopy and density functional theory calculation of graphene on a Hex-Au(001) surface. A bandgap of 0.2 eV in the graphene Dirac cone was observed at the crossing point of the graphene Dirac cone and Au 6sp bands, indicating that the origin of the bandgap formation was the hybridization between the graphene Dirac cone and Au 6sp band. We discussed the hybridization mechanism and anticipated spin injection into the graphene Dirac cone.

Journal Articles

Measurement of double-differential neutron yields for iron, lead, and bismuth induced by 107-MeV protons for research and development of accelerator-driven systems

Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta*; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.

EPJ Web of Conferences, 284, p.01023_1 - 01023_4, 2023/05

 Times Cited Count:0 Percentile:0.21(Nuclear Science & Technology)

For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron, lead, and bismuth have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics. The measured TTNYs and DDXs were compared with calculations by the Monte Carlo transport code PHITS with its default physics model of INCL version 4.6 combined with GEM and those with the JENDL-4.0/HE nuclear data library.

Journal Articles

Extreme chemistry of superheavy elements

Sato, Tetsuya; Nagame, Yuichiro*

Nihon Butsuri Gakkai-Shi, 78(2), p.64 - 72, 2023/02

The study of the chemistry of superheavy elements, which are located in the heavy extremes of the periodic table, has made considerable progress over the past 20 years, and new approaches based on various ideas have recently been developed. Research groups in Japan have also made significant contributions to the development of research on superheavy elements. Recently, notable results have been reported for the transactinide elements rutherfordium (element 104), dubnium (element 105), and seaborgium (element 106), and the heavy actinides with atomic numbers exceeding 100. The review will focus on the recent main results of these elements. This review outlines the main recent results and touches on future prospects.

Journal Articles

Band gap opening in graphene by hybridization with Au (001) reconstructed surfaces

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Physical Review Materials (Internet), 7(1), p.014002_1 - 014002_10, 2023/01

 Times Cited Count:4 Percentile:78.07(Materials Science, Multidisciplinary)

Au(001) surfaces exhibit a complex reconstructed structure [Hex-Au(001)] comprising a hexagonal surface and square bulk lattices, yielding a quasi-one-dimensional corrugated surface. When graphene was grown on this surface, the periodicity of the corrugated surface was predicted to change the electronic structure of graphene, forming bandgaps and new Dirac points. Furthermore, the graphene-Au interface is promising for bandgap generation and spin injection due to band hybridization. Here, we report the angle-resolved photoemission spectroscopy and density functional calculation of graphene on a Hex-Au(001) surface. The crossing point of the original and replica graphene $$pi$$ bands showed no bandgap, suggesting that the one-dimensional potential was too small to modify the electronic structure. A bandgap of 0.2 eV was observed at the crossing point of the graphene $$pi$$ and Au $$6sp$$ bands, indicating that the bandgap is generated using hybridization of the graphene $$pi$$ and Au $$6sp$$ bands. We discussed the hybridization mechanism and concluded that the R30 configuration between graphene and Au and an isolated electronic structure of Au are essential for effective hybridization between graphene and Au. We anticipate that hybridization between graphene $$pi$$ and Au $$6sp$$ would result in spin injection into graphene.

Journal Articles

Application of high-energy-resolution X-ray absorption spectroscopy at the U L$$_{3}$$-edge to assess the U(V) electronic structure in FeUO$$_{4}$$

Yomogida, Takumi; Akiyama, Daisuke*; Ouchi, Kazuki; Kumagai, Yuta; Higashi, Kotaro*; Kitatsuji, Yoshihiro; Kirishima, Akira*; Kawamura, Naomi*; Takahashi, Yoshio*

Inorganic Chemistry, 61(50), p.20206 - 20210, 2022/12

 Times Cited Count:4 Percentile:34.43(Chemistry, Inorganic & Nuclear)

FeUO$$_{4}$$ was studied to clarify the electronic structure of U(V) in a metal monouranate compound. We obtained the peak splitting of HERFD-XANES spectra utilizing high-energy-resolution fluorescence detection-X-ray absorption near edge structure (HERFD-XANES) spectroscopy at the U L$$_{3}$$-edge, which is a novel technique in the U(V) compounds. Theoretical calculations revealed that the peak splitting was caused by splitting the 6d orbital of U(V). Such distinctive electronic states are of major interest to researchers and engineers working in various fields, from fundamental physics to the nuclear industry and environmental sciences for actinide elements.

Journal Articles

Investigation of radioactive samples for neutron capture reaction measurements using energy-resolved neutron imaging

Segawa, Mariko; Toh, Yosuke; Kai, Tetsuya; Kimura, Atsushi; Nakamura, Shoji

Annals of Nuclear Energy, 167, p.108828_1 - 108828_5, 2022/03

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

Initial sintering kinetics of non-stoichiometric CeO$$_{2-x}$$

Watanabe, Masashi; Seki, Takayuki*

Materials Science & Engineering B, 272, p.115369_1 - 115369_6, 2021/10

 Times Cited Count:1 Percentile:7.51(Materials Science, Multidisciplinary)

The effect of oxygen non-stoichiometry on the initial sintering behavior of CeO$$_{2}$$ was investigated. It was found that the initial sintering of the stoichiometric and hypo-stoichiometric composition was controlled by the grain boundary diffusion. The activation energies of cation diffusion were derived from initial sintering data. Moreover, it is suggested that the cation diffusion was caused by a vacancy mechanism.

Journal Articles

Internal strain distribution of laser lap joints in steel under loading studied by high-energy synchrotron radiation X-rays

Shobu, Takahisa; Shiro, Ayumi*; Kono, Fumiaki*; Muramatsu, Toshiharu; Yamada, Tomonori; Naganuma, Masayuki; Ozawa, Takayuki

Quantum Beam Science (Internet), 5(2), p.17_1 - 17_9, 2021/06

The automotive industries employ laser beam welding because it realizes a high energy density without generating irradiation marks on the opposite side of the irradiated surface. Typical measurement techniques such as strain gauges and tube X-rays cannot assess the localized strain at a joint weld. Herein high-energy synchrotron radiation X-ray diffraction was used to study the internal strain distribution of laser lap joint PNC-FMS steels (2- and 5-mm thick) under loading at a high temperature. As the tensile load increased, the local tensile and compressive strains increased near the interface. These changes agreed well with the finite element analysis results. However, it is essential to complementarily utilize internal defect observations by X-ray transmission imaging because the results depend on the defects generated by laser processing.

Journal Articles

Magnetization energy current in the axial magnetic effect

Shitade, Atsuo*; Araki, Yasufumi

Physical Review B, 103(15), p.155202_1 - 155202_8, 2021/04

 Times Cited Count:2 Percentile:17.05(Materials Science, Multidisciplinary)

The axial magnetic effect (AME) is one of the anomalous transport phenomena in which the energy current is induced by an axial magnetic field. Here we numerically study the AME for the relativistic Wilson fermion in the axial magnetic field and a twisted Dirac semimetal. The AME current density inside the bulk is nonzero, and particularly in the low energy regime for the former model, it is explained by the field-theoretical results without any fitting parameter. However, for both models, the average AME current density vanishes owing to the surface contribution. The axial gauge field is regarded as the spatially modulated (effective) Zeeman field and induces the spatially modulated energy magnetization. The AME is attributed to the magnetization energy current and hence cannot be observed in transport experiments.

Journal Articles

Estimation of uncertainty in proton-induced spallation neutron multiplicity for Pb, W, Fe, and C targets

Iwamoto, Hiroki; Meigo, Shinichiro

JPS Conference Proceedings (Internet), 33, p.011046_1 - 011046_6, 2021/03

no abstracts in English

Journal Articles

The Future of energy, the challenge of "spintronics"

Ieda, Junichi

FBNews, (528), p.1 - 5, 2020/12

no abstracts in English

Journal Articles

Topics from radiation safety design of J-PARC

Nakashima, Hiroshi

JAEA-Conf 2020-001, p.69 - 74, 2020/12

J-PARC (Japan Proton Accelerator Research Complex) is a high-energy proton accelerator complex of the world's highest beam power. Because of its very high beam power and its high energy as well as the large-scale accelerator complex, we encountered some very difficult problems on radiation safety design. Various examinations and countermeasures were considered in order to overcome the difficulty. This paper introduces some of them. In addition, some new knowledge obtained during 10 years after completion are described.

Journal Articles

Low temperature heat capacity of Cs$$_{2}$$Si$$_{4}$$O$$_{9}$$

Suzuki, Eriko; Nakajima, Kunihisa; Osaka, Masahiko; Oishi, Yuji*; Muta, Hiroaki*; Kurosaki, Ken*

Journal of Nuclear Science and Technology, 57(7), p.852 - 857, 2020/07

 Times Cited Count:4 Percentile:44.4(Nuclear Science & Technology)

The low temperature heat capacity of Cs$$_{2}$$Si$$_{4}$$O$$_{9}$$, which is one of the cesium chemisorbed compounds onto stainless steel during severe accident of the light water nuclear reactor, was experimentally determined for the first time in the temperature range of 1.9 - 302 K. The experimentally determined heat capacity, $$C_{p}$$$$^{o}$$ (298.15K), and the standard entropy, $$S^{o}$$ (298.15K), were 249.4 $$pm$$ 1.1 J K$$^{-1}$$ mol$$^{-1}$$ and 322.1 $$pm$$ 1.3 J K$$^{-1}$$ mol$$^{-1}$$, respectively. The standard Gibbs energy of formation of Cs$$_{2}$$Si$$_{4}$$O$$_{9}$$ at high temperatures, $$Delta$$$$_{f}$$$$G^{o}$$($$T$$), were reevaluated by using the presently obtained $$S^{o}$$ (298.15K) and the previously reported experimental results of the standard enthalpy of formation, $$Delta$$$$_{f}$$$$H^{o}$$ (298.15K), and the standard enthalpy increments at high temperatures, $$H^{o}$$($$T$$)-$$H^{o}$$ (298.15K).

Journal Articles

Comparison of dislocation density, twin fault probability, and stacking fault energy between CrCoNi and CrCoNiFe medium entropy alloys deformed at 293 and 140K

Woo, W.*; Naeem, M.*; Jeong, J.-S.*; Lee, C.-M.*; Harjo, S.; Kawasaki, Takuro; He, H.*; Wang, X.-L.*

Materials Science & Engineering A, 781, p.139224_1 - 139224_7, 2020/04

 Times Cited Count:39 Percentile:93.25(Nanoscience & Nanotechnology)

Journal Articles

Internal residual stress evaluation of bearing balls for automobile parts

Miyakawa, Susumu*; Ito, Toshimasa*; Iwahori, Keisuke*; Aoyama, Yoshihiko*; Kubo, Ryosuke*; Murata, Shinji*; Shobu, Takahisa; Shiro, Ayumi*; Kajiwara, Kentaro*

Zairyo, 69(4), p.308 - 314, 2020/04

White etching area which looks white with nital corrosive liquid may be recognized at the flaking part of a rolling bearing on which high contact stress of several GPa is applied repeatedly. Up to now, studies of white etching area of a ball have been less than studies of white etching area of inner and outer rings. In this study, as part of the flaking mechanism explication with white etching area of a ball, internal residual stress distributions of ball by using high energy white X-ray of SPring-8 (A method) and laboratorial X-ray measurement equipment (B method) were investigated. The former was modified by surface residual stress according to B method. The latter was modified by releasing stress in the form of electrolytic polishing. The results showed modified residual stress distributions almost agree qualitatively.

Journal Articles

J-PARC H$$^{-}$$ ion source and space-charge neutralized LEBT for 100-mA high energy and high duty factor LINACs

Ueno, Akira

Review of Scientific Instruments, 91(3), p.033312_1 - 033312_9, 2020/03

 Times Cited Count:4 Percentile:27.82(Instruments & Instrumentation)

In July 2019, a 3 GeV 920 kW beam was accelerated for 10.5 hours in the J-PARC. During the operation, the H$$^{-}$$ ion source and LINAC was operated with the beam duty factor (BDF) of 1.25% (0.5 ms$$times$$25 Hz) and the ejected beam intensities of 58 and 50 mA, respectively. Separately, they were stably operated with the BDF of 1.5% (0.6 ms$$times$$25 Hz) and the ejected beam intensities of 72 and 60 mA, respectively. Based upon the 100-mA and BDF 5% (1 ms$$times$$50 Hz) H$$^{-}$$ ion source operation on a test-stand, the possibility of the 100-mA high energy and high duty factor LINACs with a radio frequency quadrupole LINAC with an injection energy higher than 64 keV is presented. The unexpectedly effective space-charge neutralization effects in the low energy beam transport are also presented. Furthermore, the transverse emittance improvements by about 8% with the shortest beam extractor are presented.

Journal Articles

Stacking fault energy analyses of additively manufactured stainless steel 316L and CrCoNi medium entropy alloy using in situ neutron diffraction

Woo, W.*; Jeong, J.-S.*; Kim, D.-K.*; Lee, C. M.*; Choi, S.-H.*; Suh, J.-Y.*; Lee, S. Y.*; Harjo, S.; Kawasaki, Takuro

Scientific Reports (Internet), 10(1), p.1350_1 - 1350_15, 2020/01

 Times Cited Count:64 Percentile:94.51(Multidisciplinary Sciences)

Journal Articles

First ionization potentials of Fm, Md, No and Lr; Verification of filling-up of 5f electrons and confirmation of the actinide series

Sato, Tetsuya

Kagaku To Kogyo, 72(10), P. 867, 2019/10

We conducted measurements of the first ionization potential (IP$$_1$$) of the heavy actinide elements, lawrencium (Lr, $$Z = 103$$), nobelium (No, $$Z = 102$$), mendelevium (Md, $$Z = 101$$) and fermium (Fm, $$Z = 100$$) by using a novel method based on a surface ionization process. The IP$$_1$$ measurements have been performed using the ISOL (Isotope Separator On-Line) system equipped with a surface ion-source with short-lived heavy actinide isotopes, $$^{256}$$Lr ($$T_{1/2}$$ = 27s), $$^{257}$$No ($$T_{1/2}$$ = 24.5s), $$^{251}$$Md ($$T_{1/2}$$ = 4.27 min), and $$^{249}$$Fm ($$T_{1/2}$$ = 2.6 min). Our experimental results clearly showed that the IP$$_1$$ of Lr is distinctly low among actinide elements. Moreover, No has the highest IP$$_1$$ among them due to its full-filled 5f and 7s orbitals; the IP$$_1$$ value increased with an atomic number up to No and decreased dramatically at Lr, indicating the similar trend with that of heavy lanthanide elements. Therefore, we concluded Lr would be the last member of the actinide series.

1014 (Records 1-20 displayed on this page)